{"id":1208,"date":"2021-01-25T20:37:42","date_gmt":"2021-01-25T11:37:42","guid":{"rendered":"http:\/\/tuat-chemphys.net\/?p=1208"},"modified":"2026-04-19T16:07:11","modified_gmt":"2026-04-19T07:07:11","slug":"%e5%bc%b7%e3%81%84%e5%8f%8d%e5%bc%b7%e7%a3%81%e6%80%a7%e4%bd%93%e3%81%ae%e3%83%a1%e3%82%bf%e3%82%bb%e3%82%b7%e3%82%b9%e5%8f%8d%e5%bf%9c-metathesis-reaction-of-unique-antiferromagnetic-material","status":"publish","type":"post","link":"https:\/\/tuat-chemphys.net\/?p=1208","title":{"rendered":"\u30e1\u30bf\u30bb\u30b7\u30b9\u53cd\u5fdc\u3092\u7528\u3044\u305f\u53cd\u5f37\u78c1\u6027\u4f53\u306e\u958b\u767a\uff08\u65b0\u7d20\u6750\u5275\u88fd\uff09&#8221;Unique&#8221; antiferromagnetic material via metathesis reaction. \u6587\u8cac: 2\u5e74\u751fM.R."},"content":{"rendered":"\n<p>\u53cd\u5f37\u78c1\u6027\u4f53\u304c\u30b9\u30d4\u30f3\u30c8\u30ed\u30cb\u30af\u30b9\u306b\u304a\u3044\u3066\u65b0\u305f\u306a\u6a5f\u80fd\u6750\u6599\u306b\u671b\u307e\u3057\u3044\u3068\u8003\u3048\u3089\u308c\u3066\u3044\u308b\u3002<\/p>\n\n\n\n<p>\u539f\u53e3\u7950\u54c9\u52a9\u6559\u3068\u9999\u53d6\u6d69\u5b50\u6559\u6388\u306f\u3001Ir<sup>4+<\/sup>\u30a4\u30aa\u30f3\u306b\u3088\u3063\u3066\u3064\u304f\u3089\u308c\u308b\u30cf\u30cb\u30ab\u30e0\u69cb\u9020\u3092\u3082\u3063\u305f\u30a4\u30eb\u30e1\u30ca\u30a4\u30c8\u578b\u306e\u30a4\u30ea\u30b8\u30a6\u30e0\u9178\u5316\u7269CdIrO<sub>3<\/sub>\u306e\u5408\u6210\u306b\u6210\u529f\u3057\u3001\u305d\u306e\u6750\u6599\u306e\u78c1\u6c17\u7279\u6027\u3092\u8abf\u3079\u305f\u3002\u6e2c\u5b9a\u306e\u7d50\u679c\u3067\u306f\u3001\u5927\u304d\u306a<strong>\u6709\u52b9\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\uff08\u78c1\u6c17\u80fd\u7387\uff09<\/strong>\u3068<strong>\u5f37\u3044\u53cd\u5f37\u78c1\u6027\u76f8\u4e92\u4f5c\u7528<\/strong>\u304c\u307f\u3089\u308c\u3066\u3001<strong>\u901a\u5e38\u306eKitaev\u30e2\u30c7\u30eb\u304b\u3089\u306e\u30ba\u30ec<\/strong>\u304c\u78ba\u8a8d\u3055\u308c\u305f\u3002<\/p>\n\n\n\n<div class=\"wp-block-image\"><figure class=\"aligncenter size-large\"><img data-recalc-dims=\"1\" loading=\"lazy\" decoding=\"async\" width=\"500\" height=\"439\" data-attachment-id=\"1209\" data-permalink=\"https:\/\/tuat-chemphys.net\/?attachment_id=1209\" data-orig-file=\"https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/%E9%A6%99%E5%8F%96%E6%B5%A9%E5%AD%90%E7%A0%94%E7%A9%B6%E5%AE%A4_%E6%8C%BF%E5%85%A5%E7%94%BB%E5%83%8F.png?fit=500%2C439&amp;ssl=1\" data-orig-size=\"500,439\" data-comments-opened=\"1\" data-image-meta=\"{&quot;aperture&quot;:&quot;0&quot;,&quot;credit&quot;:&quot;&quot;,&quot;camera&quot;:&quot;&quot;,&quot;caption&quot;:&quot;&quot;,&quot;created_timestamp&quot;:&quot;0&quot;,&quot;copyright&quot;:&quot;&quot;,&quot;focal_length&quot;:&quot;0&quot;,&quot;iso&quot;:&quot;0&quot;,&quot;shutter_speed&quot;:&quot;0&quot;,&quot;title&quot;:&quot;&quot;,&quot;orientation&quot;:&quot;0&quot;}\" data-image-title=\"\u9999\u53d6\u6d69\u5b50\u7814\u7a76\u5ba4_\u633f\u5165\u753b\u50cf\" data-image-description=\"\" data-image-caption=\"\" data-large-file=\"https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/%E9%A6%99%E5%8F%96%E6%B5%A9%E5%AD%90%E7%A0%94%E7%A9%B6%E5%AE%A4_%E6%8C%BF%E5%85%A5%E7%94%BB%E5%83%8F.png?fit=500%2C439&amp;ssl=1\" src=\"https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/%E9%A6%99%E5%8F%96%E6%B5%A9%E5%AD%90%E7%A0%94%E7%A9%B6%E5%AE%A4_%E6%8C%BF%E5%85%A5%E7%94%BB%E5%83%8F.png?resize=500%2C439&#038;ssl=1\" alt=\"\" class=\"wp-image-1209\" srcset=\"https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/%E9%A6%99%E5%8F%96%E6%B5%A9%E5%AD%90%E7%A0%94%E7%A9%B6%E5%AE%A4_%E6%8C%BF%E5%85%A5%E7%94%BB%E5%83%8F.png?w=500&amp;ssl=1 500w, https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/%E9%A6%99%E5%8F%96%E6%B5%A9%E5%AD%90%E7%A0%94%E7%A9%B6%E5%AE%A4_%E6%8C%BF%E5%85%A5%E7%94%BB%E5%83%8F.png?resize=300%2C263&amp;ssl=1 300w\" sizes=\"auto, (max-width: 500px) 100vw, 500px\" \/><figcaption>CdIrO3\u306e\u7d50\u6676\u69cb\u9020\u3000Crystal structure of&nbsp;CdIrO3&nbsp;(a) viewed along the&nbsp;c&nbsp;axis and (b) perpendicular to the&nbsp;ab&nbsp;plane. (c) The local environment of a pair of edge-sharing&nbsp;IrO6&nbsp;octahedra with the two different bond lengths of Ir-O and the bond angle of Ir-O-Ir.&nbsp;<\/figcaption><\/figure><\/div>\n\n\n\n<p>\u516b\u9762\u4f53IrO<sub>6<\/sub>\u306e\u30e1\u30bf\u30bb\u30b7\u30b9\u7684\u306b\u5b89\u5b9a\u5316\u3055\u308c\u305f\u5927\u304d\u306a\u4e09\u89d2\u6b6a\u307f\u306e\u305f\u3081\u3001CdIrO<sub>3<\/sub>\u306e\u7d76\u7e01\u4f53\u72b6\u614b\u306f\u5f93\u6765\u306eIr<sup>4+<\/sup>\u30a4\u30aa\u30f3\u3067\u30a4\u30aa\u30f3\u3067\u671f\u5f85\u3055\u308c\u3066\u3044\u308b\u96fb\u5b50\u72b6\u614b\uff08<em>J<sub>eff<\/sub><\/em> =1\/2\u30e2\u30c3\u30c8\u72b6\u614b\uff09\u3067\u306f\u8aac\u660e\u3067\u304d\u306a\u3044\u3002CdIrO<sub>3<\/sub>\u304c\u8208\u5473\u6df1\u3044\u300c<strong>\u53cd\u5f37\u78c1\u6027\u4f53\u300d<\/strong>\u3068\u306a\u308a\u3001\u3055\u3089\u306a\u308b\u5c55\u958b\u304c\u671f\u5f85\u3055\u308c\u308b\u3002<\/p>\n\n\n\n<p>Dr. Yuya Haraguchi and Prof. Hiroko Katori have successfully synthesized a metastable honeycomb lattice iridate CdIrO3 with an ilmenite structure via <strong>a metathesis reaction<\/strong> and investigated its crystal structure and magnetism.<\/p>\n\n\n\n<p>The magnetization measurements indicated a large effective magnetic moment and a fairly strong antiferromagnetic interaction, which indicated a deviation from the &#8220;conventional&#8221; Kitaev model. Also, insulating CdIrO<sub>3<\/sub> cannot be described as a \u201ctypical\u201c state (<em>J<sub>eff <\/sub><\/em>=1\/2 Mott state) owing to a metathetically stabilized large trigonal distortion of IrO<sub>6<\/sub> octahedra.&nbsp;<\/p>\n\n\n\n<p>CdIrO<sub>3<\/sub> has become an interesting antiferromagnetic material and further developments are expected.<\/p>\n\n\n\n<p><\/p>\n\n\n\n<p>\u6587\u8cac: #\u5316\u5b66\u7269\u7406\u5de5\u5b66\u79d12\u5e74\u751f M.R.<\/p>\n\n\n\n<p><strong>Reference:<\/strong> Strong antiferromagnetic interaction owing to a large trigonal distortion in the spin-orbit-coupled honeycomb lattice iridate CdIrO3 (<a href=\"https:\/\/researchmap.jp\/chiyuya\" target=\"_blank\" rel=\"noreferrer noopener\">Yuya Haraguchi<\/a> &amp; <a href=\"https:\/\/researchmap.jp\/read0117904\/\" target=\"_blank\" rel=\"noreferrer noopener\">Hiroko Aruga-Katori<\/a>) <strong><em>Phys. Rev. Materials<\/em><\/strong> (2020) <strong>American Physical Society<\/strong>\u30a2\u30e1\u30ea\u30ab\u7269\u7406\u5b66\u4f1a <a rel=\"noreferrer noopener\" href=\"https:\/\/doi.org\/10.1103\/PhysRevMaterials.4.044401\" target=\"_blank\"><strong>doi.org\/10.1103\/PhysRevMaterials.4.044401<\/strong><\/a><\/p>\n\n\n\n<p><\/p>\n\n\n\n<p class=\"has-text-align-center\"><strong>\u3010\u7528\u8a9e\u3011<\/strong><\/p>\n\n\n\n<p><strong>\u53cd\u5f37\u78c1\u6027\u76f8\u4e92\u4f5c\u7528<\/strong>\uff1a\u78c1\u6027\u30a4\u30aa\u30f3\u304c\u6301\u3064\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\u306e\u9593\u306b\u50cd\u304f\u76f8\u4e92\u4f5c\u7528\u306e\u3046\u3061\u3001\u96a3\u3044\u5408\u3046\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\u3092\u53cd\u5bfe\u65b9\u5411\u306b\u914d\u5217\u3055\u305b\u308b\u76f8\u4e92\u4f5c\u7528\u306e\u3053\u3068\u3002<\/p>\n\n\n\n<p><strong>\u53cd\u5f37\u78c1\u6027\u4f53\uff1a<\/strong>\u53cd\u5f37\u78c1\u6027\u76f8\u4e92\u4f5c\u7528\u306b\u3088\u308a\u96a3\u308a\u5408\u3046\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\u304c\u53cd\u5bfe\u65b9\u5411\u3092\u5411\u3044\u3066\u914d\u5217\u3057\u3066\u304a\u308a\u3001\u6c38\u4e45\u78c1\u77f3\u3067\u767a\u751f\u3067\u304d\u308b\u5f37\u3055\u306e\u5916\u90e8\u78c1\u5834\u306b\u5bfe\u3057\u3066\u3082\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\u306e\u914d\u5217\u306f\u307b\u3068\u3093\u3069\u5909\u5316\u3057\u306a\u3044\u3002\u4f8b\u3048\u3070\u3001\u53cd\u5f37\u78c1\u6027\u4f53\u306e\u6027\u8cea\u3092\u5229\u7528\u3059\u308b\u3053\u3068\u3067\u3001\u78c1\u6c17\u30e2\u30fc\u30e1\u30f3\u30c8\u306e\u56de\u8ee2\uff08\u96fb\u6d41\u3067\u66f8\u304d\u8fbc\u307f\uff09\u304c\u3067\u304d\u308b\u304c\u3001\u5916\u90e8\u78c1\u5834\u64fe\u4e71\u306b\u306f \u5f37\u3044\u78c1\u6c17\u30e1\u30e2\u30ea\u304c\u5b9f\u73fe\u3067\u304d\u308b\u53ef\u80fd\u6027\u304c\u3042\u308b\u3002<\/p>\n\n\n\n<p><strong>Kitaev model<\/strong> = \u7570\u65b9\u7684\u76f8\u4e92\u4f5c\u7528\u3092\u3082\u3064\u300c\u91cf\u5b50\u30b3\u30f3\u30d1\u30b9\u6a21\u578b\u300d\u304c\u30cf\u30cb\u30ab\u30e0\u683c\u5b50\u4e0a\u3067\u306f\u53b3\u5bc6\u89e3\u3068\u3057\u3066\u91cf\u5b50\u30b9\u30d4\u30f3\u6db2\u4f53\u3068\u306a\u308b\u30e2\u30c7\u30eb\uff08Kitaev\u6c0f\u306b\u3088\u3063\u3066\u63d0\u6848\u3055\u308c\u305f\uff09<\/p>\n\n\n\n<p><strong>\u30e2\u30c3\u30c8\u7d76\u7e01\u4f53<\/strong> (<strong>Mott-insulator)<\/strong> \uff1d\u3000\u30d0\u30f3\u30c9\u7406\u8ad6\u3067\u306f\u91d1\u5c5e\u7684\u3068\u4e88\u60f3\u3055\u308c\u308b\u306b\u3082\u304b\u304b\u308f\u3089\u305a\u3001\u96fb\u5b50\u9593\u65a5\u529b\u306e\u52b9\u679c\uff08\u96fb\u5b50\u76f8\u95a2\u52b9\u679c\uff09\u306b\u3088\u3063\u3066\u5b9f\u73fe\u3057\u3066\u3044\u308b<strong>\u7d76\u7e01\u4f53<\/strong>\u72b6\u614b\u306e\u3053\u3068\u3002<\/p>\n\n\n\n<p><strong>Metathesis reactions =<\/strong>&nbsp;Chemical&nbsp;<strong>reactions<\/strong>&nbsp;in which two hydrocarbons (alkanes, alkenes or alkynes) are converted to two new hydrocarbons by the exchange of carbon\u2013carbon single, double or triple bonds.&nbsp;<\/p>\n\n\n\n<p><\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u5408\u6210\u3055\u308c\u305f\u300c\u8208\u5473\u6df1\u3044\u300d\u53cd\u5f37\u78c1\u6027\u4f53\u304c\u30b9\u30d4\u30f3\u30c8\u30ed\u30cb\u30af\u30b9\u306b\u304a\u3044\u3066\u65b0\u305f\u306a\u6a5f\u80fd\u6750\u6599\u306b\u671b\u307e\u3057\u3044\u3068\u8003\u3048\u3089\u308c\u3066\u3044\u308b\u3002Interesting\/unique antiferromagnetic materials are considered to be desirable for new functional materials in spintronics.<\/p>\n","protected":false},"author":2,"featured_media":1210,"comment_status":"closed","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"advanced_seo_description":"","jetpack_seo_html_title":"","jetpack_seo_noindex":false,"jetpack_post_was_ever_published":false,"_jetpack_newsletter_access":"","_jetpack_dont_email_post_to_subs":false,"_jetpack_newsletter_tier_id":0,"_jetpack_memberships_contains_paywalled_content":false,"_jetpack_memberships_contains_paid_content":false,"footnotes":"","jetpack_publicize_message":"","jetpack_publicize_feature_enabled":true,"jetpack_social_post_already_shared":true,"jetpack_social_options":{"image_generator_settings":{"template":"highway","default_image_id":0,"font":"","enabled":false},"version":2}},"categories":[9],"tags":[14,27],"class_list":["post-1208","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-research","tag-advanced-materials-creation","tag-quantum-tech"],"jetpack_publicize_connections":[],"jetpack_featured_media_url":"https:\/\/i0.wp.com\/tuat-chemphys.net\/wp-content\/uploads\/2021\/01\/pexels-photo-6429127.jpeg?fit=1880%2C1253&ssl=1","jetpack_sharing_enabled":true,"jetpack-related-posts":[{"id":6462,"url":"https:\/\/tuat-chemphys.net\/?p=6462","url_meta":{"origin":1208,"position":0},"title":"\u4fee\u58eb\u5b66\u751f\u304c\u6311\u3080 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